The Library of the Monastery it was founded by Hosios Christodoulos, who, it is said, procured the first books. Today the Library possesses a quantity of 900 manuscripts among which the 325 are written over parchments. It exist also more than 2000 volumes of ancient editions and 13000 copies of various documents. A catalogue of these books was authored by John Sakelion, which book appeared in the year 1890. The catalogue was later completed by the Deacon Callimachus. Among the most important manuscripts we must name the following : the manuscript of Diodore Sikeliotis, the Purple Code, an incomplete copy of Evangelist Mark’s Gospel, the book of Job, manuscripts of the 7th and 8th century AD, sermons of St. Gregory the Theologue, the Gospel of Four – a manuscript dated from 1345 AD – which contains very beautiful images of the Evangelists, 29 roll manuscripts on parchments containing the test of Messes written of St.Basile the Great and St.John the Chrysostome and many other of several prelates, the Glossarion (vocabulary), which is a dictionary of the Greek language written on parchment, the did of gift of Emperor Alexios Comninos I, by which this Sovereign donated the island of Patmos to Hosios Christodoulos. Finally there exist a lot of documents of the Byzance Emperors, the Patriarchs, the Princes and other Dignitaries.
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